Fast-neutron inelastic scattering cross sections for the principal even-even actinide nuclei. III. <sup>240,242,244</sup>Pu(n,n')
E Sheldon; D W S Chan; E Sheldon; Dept. of Phys. & Appl. Phys., Lowell Univ., MA, USA; D W S Chan; Dept. of Phys. & Appl. Phys., Lowell Univ., MA, USA
Журнал:
Journal of Physics G: Nuclear Physics
Дата:
1987-02-01
Аннотация:
For pt.II see ibid., vol.12, p.443, 1986. The review of fast-neutron inelastic scattering data for the principal even-even actinide nuclei, as undertaken previously for <sup>232</sup>Th(n,n') and <sup>238</sup>U(n,n') level excitation functions and angular distributions, is here continued for <sup>240,242,244</sup>Pu(n,n') from threshold to 2.5 or 3.5 MeV. Differential and total (angle-integrated) cross sections have been calculated on the basis of proposed collective-band level schemes in the 'standard' (CN+DI) formalism and in the statistical S-matrix formalism of Hofmann, Richert, Tepel and Weidenmuller (the HRTW approach). For consistency throughout, the optical potential and deformation parameters have followed the Bruyeres prescription, except that for <sup>244</sup>Pu Nilsson harmonic-oscillator deformation parameters were chosen. Corrections were applied to the compound-nucleus (CN) cross sections to take account of Moldauer level-width fluctuations, extra n'-channel and radiative-capture competition; for <sup>240,242</sup>Pu+n, fission competition was also taken into account and for <sup>242,244</sup>Pu+n, provision for continuum competition was also made. So far as possible, theoretical data were compared with (the sparse and somewhat unreliable) experimental results and with the ENDF/B-V evaluation: for <sup>240</sup>Pu(n,n') the only available measured data were level excitation functions to E<sub>n</sub>=1.5 MeV for the 2<sup>+</sup>, 4<sup>+</sup> and 6<sup>+</sup> states in the ground-state rotational band and for grouped 'composite' vibrational levels; for <sup>242</sup>Pu(n,n') the experimental excitation function and angular distribution data extended to E<sub>n</sub>=3.4 MeV for the 2<sup>+</sup> and 4<sup>+</sup> rotational states; no data existed for <sup>244</sup>Pu(n,n'). The body of calculated cross-section data thus serves as a comprehensive database for the primary rotational and vibrational states in the three principal even-mass fertile Pu isotopes, wherein the HRTW angle-integrated values demonstrate the viability of this as yet underexploited method.
1.408Мб