Competitive contributions of short-range magnetic order and chemical disorder to the resistivity in Co<sub>30</sub>Pt<sub>70</sub>
C Leroux; M C Cadeville; R Kozubski; C Leroux; Inst. de Phys. et Chimie des Mater. de Strasbourg, CNRS, France; M C Cadeville; Inst. de Phys. et Chimie des Mater. de Strasbourg, CNRS, France; R Kozubski; Inst. de Phys. et Chimie des Mater. de Strasbourg, CNRS, France
Журнал:
Journal of Physics: Condensed Matter
Дата:
1989-09-11
Аннотация:
A comparative study of the dependence on T of the resistivity in non-magnetic Ni<sub>30</sub>Pt<sub>70</sub> and paramagnetic Co<sub>30</sub>Pt<sub>70</sub> alloys in their ordered (L1<sub>2</sub>-type structure) and disordered (A<sub>1</sub>) phase is presented. In order to make measurements of as far as possible real thermodynamic equilibrium states, the heating rates were chosen taking into account previous (Co<sub>30</sub>Pt<sub>70</sub>) or present (Ni<sub>30</sub>Pt<sub>70</sub>) order kinetics data. The authors find that in Ni<sub>30</sub>Pt<sub>70</sub> the resistivity can be analysed in terms of two main contributions: (i) a term of 4 K residual resistivity associated with the chemical disorder, and its variation with T, which is separately measured using a specific device; and (ii) a phonon-like term, proportional to T. In Co<sub>30</sub>Pt<sub>70</sub>, a further term associated with the spin-disorder scattering at present. In the paramagnetic range, this term decreases with T as the chemical disorder increases, the decrease being especially large at the order-disorder (L1<sub>2</sub>-A<sub>1</sub>) transition. Such behaviour is attributed to the existence of short-range magnetic order in the paramagnetic state of Co<sub>30</sub>Pt<sub>70</sub>, which would be enhanced by the increase of the chemical disorder, i.e. by the increase of the Co-Co coordination, thus reducing the spin-disorder contribution to the resistivity. All the data are in very good agreement with a previous comparative study of equi-atomic NiPt and CoPt phases, which led to a similar conclusion.
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