Автор |
A Krimmel |
Автор |
J Hemberger |
Автор |
C Kegler |
Автор |
M Nicklas |
Автор |
A Engelmayer |
Автор |
G Knebel |
Автор |
V Fritsch |
Автор |
M Reehuis |
Автор |
M Brando |
Автор |
A Loidl |
Дата выпуска |
1999-09-13 |
dc.description |
We have studied the magnetic behaviour of PrAu<sub>2</sub>(Si<sub>1-x</sub>Ge<sub>x</sub>)<sub>2</sub> by means of magnetic susceptibility, resistivity, and heat capacity measurements, and x-ray and neutron powder diffraction. All compounds are isostructural and crystallize in the well known ThCr<sub>2</sub>Si<sub>2</sub>-type structure. PrAu<sub>2</sub>Si<sub>2</sub> shows the characteristic features of a canonical spin glass with a freezing temperature of T<sub>F</sub> = 3 K. Completely unexpectedly, on introducing/increasing the atomic disorder by alloying with Ge, the spin-glass transition is suppressed as is first evident from a slight decrease of the freezing temperature T<sub>F</sub> up to x = 0.10. Long-range magnetic order sets in for x0.12. Within the range 0.15 x1, all compounds show the same simple AF-I-type antiferromagnetic structure with a monotonic increase of both the Néel temperature and the ordered magnetic moment for increasing Ge concentration. The magnetic phase diagram of PrAu<sub>2</sub>(Si<sub>1-x</sub>Ge<sub>x</sub>)<sub>2</sub> is explained by the presence of weak disorder at a constant level at the Au sites. Clear indications of crystal-field effects have been observed. |
Формат |
application.pdf |
Издатель |
Institute of Physics Publishing |
Название |
The evolution from long-range magnetic order to spin-glass behaviour in PrAu<sub>2</sub>(Si<sub>1-x</sub>Ge<sub>x</sub>)<sub>2</sub> |
Тип |
paper |
DOI |
10.1088/0953-8984/11/36/315 |
Electronic ISSN |
1361-648X |
Print ISSN |
0953-8984 |
Журнал |
Journal of Physics: Condensed Matter |
Том |
11 |
Первая страница |
6991 |
Последняя страница |
7003 |
Аффилиация |
A Krimmel; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Аффилиация |
J Hemberger; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Аффилиация |
C Kegler; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Аффилиация |
M Nicklas; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Аффилиация |
A Engelmayer; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Аффилиация |
G Knebel; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Аффилиация |
V Fritsch; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Аффилиация |
M Reehuis; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Аффилиация |
M Brando; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Аффилиация |
A Loidl; Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, D-86159 Augsburg, Germany |
Выпуск |
36 |