Автор |
I O Troyanchuk |
Автор |
D D Khalyavin |
Автор |
S V Trukhanov |
Автор |
H Szymczak |
Дата выпуска |
1999-11-08 |
dc.description |
The magnetization and magnetoresistance of Ln<sub>1-x</sub>Ba<sub>x</sub>MnO<sub>3</sub> have been studied for a single crystal (Ln = Nd, x = 0.23) and for ceramics (Ln = Nd, Sm; 0 x0.44). It was shown that Nd<sub>1-x</sub>Ba<sub>x</sub>MnO<sub>3</sub> compositions in the range 0 x0.05 are inhomogeneous antiferromagnets; a mixed antiferro-ferromagnet state appears in the range 0.05<x<0.10; a pure ferromagnetic state develops in the range 0.2 x<0.4 and in the range x0.4 an inhomogeneous ferromagnetic state is realized. Metal-like behaviour below T<sub>C</sub> is found in the concentration 0.3<x0.44. The concentrational transition from inhomogeneous antiferromagnetic state into spin-glass state in Sm<sub>1-x</sub>Ba<sub>x</sub>MnO<sub>3</sub> was found at x>0.12. Both Nd and Sm sublattices are coupled antiferromagnetically with manganese ions. All the ferromagnetic Nd<sub>1-x</sub>Ba<sub>x</sub>MnO<sub>3</sub> samples show similar magnetotransport properties despite of a strong difference in the resistivity behaviour. Our results could be understood in terms of Mn-O-Mn superexchange and 3d orbital ordering as well as variation of band structure due to the ionic size effect, Mn<sup>4+</sup> ion appearance and magnetic ordering. It is supposed that the gap between the narrow 3d manganese band and wide 2p oxygen band decreases strongly below T<sub>C</sub>. |
Формат |
application.pdf |
Издатель |
Institute of Physics Publishing |
Название |
Magnetic phase diagrams of the manganites Ln<sub>1-x</sub>Ba<sub>x</sub>MnO<sub>3</sub> (Ln = Nd, Sm) |
Тип |
paper |
DOI |
10.1088/0953-8984/11/44/309 |
Electronic ISSN |
1361-648X |
Print ISSN |
0953-8984 |
Журнал |
Journal of Physics: Condensed Matter |
Том |
11 |
Первая страница |
8707 |
Последняя страница |
8717 |
Выпуск |
44 |