Автор |
Vadim A Markel |
Автор |
Michael R Geller |
Дата выпуска |
2000-08-28 |
dc.description |
There is currently great interest in the dynamics of electrons and phonons in low-dimensional systems, where the effects of quantum confinement cause a dramatic difference in their behaviour as compared with bulk systems. In this paper we consider a localized electronic impurity state (an electronic two-level system) linearly coupled to the vibrational modes of an isolated nanometre-scale insulating crystal, and study the phonon emission rate at frequencies less than that of the lowest internal vibrational mode, i.e., in the acoustic `gap'. We show that, at finite temperature, electronic energy relaxation below the acoustic gap can occur as a result of anharmonic broadening of vibrational modes, and we calculate the frequency and temperature dependence of the relaxation provided by this mechanism. |
Формат |
application.pdf |
Издатель |
Institute of Physics Publishing |
Название |
One-phonon relaxation of localized electronic states in anharmonic nanoparticles |
Тип |
paper |
DOI |
10.1088/0953-8984/12/34/304 |
Electronic ISSN |
1361-648X |
Print ISSN |
0953-8984 |
Журнал |
Journal of Physics: Condensed Matter |
Том |
12 |
Первая страница |
7569 |
Последняя страница |
7582 |
Аффилиация |
Vadim A Markel; Department of Physics and Astronomy, University of Georgia, Athens, GA 30602-2451, USA |
Аффилиация |
Michael R Geller; Department of Physics and Astronomy, University of Georgia, Athens, GA 30602-2451, USA |
Выпуск |
34 |