Small-signal dielectric relaxation in the disordered perovskite Pb(Mg<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub>
H M Christen; R Sommer; N K Yushin; J J van der Klink; H M Christen; Inst. de Phys. Exp., Ecole Polytech. Federale de Lausanne, Switzerland; R Sommer; Inst. de Phys. Exp., Ecole Polytech. Federale de Lausanne, Switzerland; N K Yushin; Inst. de Phys. Exp., Ecole Polytech. Federale de Lausanne, Switzerland; J J van der Klink; Inst. de Phys. Exp., Ecole Polytech. Federale de Lausanne, Switzerland
Журнал:
Journal of Physics: Condensed Matter
Дата:
1994-03-28
Аннотация:
Decay-current and conventional dielectric measurements have been performed on single-crystal samples of the disordered perovskite Pb(Mg<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub>(PMN). Low-frequency dielectric data of Colla and co-workers(1992) on the same system are critically reanalysed and compared to our results. In contrast to previously proposed spin-glass or master-plot approaches, we suggest a phenomenological description in terms of alpha - and beta -relaxations: a relatively high-frequency beta -process takes over when the characteristic alpha -relaxation time becomes extremely long. The continuous slowing down of polar motion distinguishes PMN from related compounds such as Pb(Zn<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub> for which, in contrast to PMN, there is evidence of astructural phase transition.
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