Low-temperature growth of thin Pb layers and the quantum size effect
D Schmicker; T Hibma; K A Edwards; P B Howes; J E MacDonald; M A James; M Breeman; G T Barkema
Журнал:
Journal of Physics: Condensed Matter
Дата:
1997-02-03
Аннотация:
It is argued that the growth morphology of ultrathin metal films should fluctuate as a function of film thickness due to the quantum size effect. To verify this, the specularly reflected intensity of x-rays, electrons and He atoms has been measured during the growth of a thin Pb layer on top of an substrate at 100 K. Curiously enough, the expected variation is observed in the He atom and electron scattering data, but not in the x-ray reflectivity. Our explanation is that the differences in the heat of formation for successive atomic layers have a strong effect on the step density, but not on the occupancy of the layers at the low growth temperatures necessary to obtain layer-by-layer growth. This is backed up by the results of a Monte Carlo simulation.
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