Far-infrared properties of two-level systems in amorphous ice
N. I. Agladze; A. J. Sievers; N. I. Agladze; Laboratory of Atomic and Solid State Physics and the Center for Radiophysics and Space Research, Cornell University - Ithaca, NY 14853-2501, USA; A. J. Sievers; Laboratory of Atomic and Solid State Physics and the Center for Radiophysics and Space Research, Cornell University - Ithaca, NY 14853-2501, USA
Журнал:
EPL (Europhysics Letters)
Дата:
2001-01-01
Аннотация:
Isotopic substitution and defect doping have been used to alter the optical properties of two-level systems (TLS) in the two amorphous phases of a-H<sub>2</sub>O ice. A large TLS optical density of states is found for a-H<sub>2</sub>O and a-HOD in the high-density amorphous phase while a thirty times smaller value occurs for both in the low-density amorphous one. Our quantitative spectroscopic and thermal study bring out a number of new features, among them that LiCl doping of low-density amorphous ice increases its TLS optical density of states, its glass transition temperature and its fragility.
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