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Автор de la Cruz, Clarina
Автор Huang, Q.
Автор Lynn, J. W.
Автор Li, Jiying
Автор II, W. Ratcliff
Автор Zarestky, J. L.
Автор Mook, H. A.
Автор Chen, G. F.
Автор Luo, J. L.
Автор Wang, N. L.
Автор Dai, Pengcheng
Дата выпуска 2008
dc.description Following the discovery of long-range antiferromagnetic order in the parent compounds of high-transition-temperature (high-Tc) copper oxides, there have been efforts to understand the role of magnetism in the superconductivity that occurs when mobile â electronsâ or â holesâ are doped into the antiferromagnetic parent compounds. Superconductivity in the newly discovered rare-earth iron-based oxide systems ROFeAs (R, rare-earth metal) also arises from either electron or hole doping of their non-superconducting parent compounds. The parent material LaOFeAs is metallic but shows anomalies near 150â K in both resistivity and d.c. magnetic susceptibility. Although optical conductivity and theoretical calculations suggest that LaOFeAs exhibits a spin-density-wave (SDW) instability that is suppressed by doping with electrons to induce superconductivity, there has been no direct evidence of SDW order. Here we report neutron-scattering experiments that demonstrate that LaOFeAs undergoes an abrupt structural distortion below 155â K, changing the symmetry from tetragonal (space group P4/nmm) to monoclinic (space group P112/n) at low temperatures, and then, at â ¼137â K, develops long-range SDW-type antiferromagnetic order with a small moment but simple magnetic structure. Doping the system with fluorine suppresses both the magnetic order and the structural distortion in favour of superconductivity. Therefore, like high-Tc copper oxides, the superconducting regime in these iron-based materials occurs in close proximity to a long-range-ordered antiferromagnetic ground state.
Формат application.pdf
Издатель Nature Publishing Group
Копирайт Nature Publishing Group
Название Magnetic order close to superconductivity in the iron-based layered LaO1-xFxFeAs systems
Тип LETTERS TO NATURE
DOI 10.1038/nature07057
Print ISSN 0028-0836
Журнал Nature
Том 453
Первая страница 899
Последняя страница 902
Аффилиация de la Cruz, Clarina; Department of Physics and Astronomy, The University of Tennessee, Knoxville, Tennessee 37996-1200, USA; Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA
Аффилиация Huang, Q.; NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, USA
Аффилиация Lynn, J. W.; NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, USA
Аффилиация Li, Jiying; NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, USA; Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742-6393, USA
Аффилиация II, W. Ratcliff; NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, USA
Аффилиация Zarestky, J. L.; Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, USA
Аффилиация Mook, H. A.; Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA
Аффилиация Chen, G. F.; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China
Аффилиация Luo, J. L.; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China
Аффилиация Wang, N. L.; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China
Аффилиация Dai, Pengcheng; Department of Physics and Astronomy, The University of Tennessee, Knoxville, Tennessee 37996-1200, USA; Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA
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