Автор |
de la Cruz, Clarina |
Автор |
Huang, Q. |
Автор |
Lynn, J. W. |
Автор |
Li, Jiying |
Автор |
II, W. Ratcliff |
Автор |
Zarestky, J. L. |
Автор |
Mook, H. A. |
Автор |
Chen, G. F. |
Автор |
Luo, J. L. |
Автор |
Wang, N. L. |
Автор |
Dai, Pengcheng |
Дата выпуска |
2008 |
dc.description |
Following the discovery of long-range antiferromagnetic order in the parent compounds of high-transition-temperature (high-Tc) copper oxides, there have been efforts to understand the role of magnetism in the superconductivity that occurs when mobile â electronsâ or â holesâ are doped into the antiferromagnetic parent compounds. Superconductivity in the newly discovered rare-earth iron-based oxide systems ROFeAs (R, rare-earth metal) also arises from either electron or hole doping of their non-superconducting parent compounds. The parent material LaOFeAs is metallic but shows anomalies near 150â K in both resistivity and d.c. magnetic susceptibility. Although optical conductivity and theoretical calculations suggest that LaOFeAs exhibits a spin-density-wave (SDW) instability that is suppressed by doping with electrons to induce superconductivity, there has been no direct evidence of SDW order. Here we report neutron-scattering experiments that demonstrate that LaOFeAs undergoes an abrupt structural distortion below 155â K, changing the symmetry from tetragonal (space group P4/nmm) to monoclinic (space group P112/n) at low temperatures, and then, at â ¼137â K, develops long-range SDW-type antiferromagnetic order with a small moment but simple magnetic structure. Doping the system with fluorine suppresses both the magnetic order and the structural distortion in favour of superconductivity. Therefore, like high-Tc copper oxides, the superconducting regime in these iron-based materials occurs in close proximity to a long-range-ordered antiferromagnetic ground state. |
Формат |
application.pdf |
Издатель |
Nature Publishing Group |
Копирайт |
Nature Publishing Group |
Название |
Magnetic order close to superconductivity in the iron-based layered LaO1-xFxFeAs systems |
Тип |
LETTERS TO NATURE |
DOI |
10.1038/nature07057 |
Print ISSN |
0028-0836 |
Журнал |
Nature |
Том |
453 |
Первая страница |
899 |
Последняя страница |
902 |
Аффилиация |
de la Cruz, Clarina; Department of Physics and Astronomy, The University of Tennessee, Knoxville, Tennessee 37996-1200, USA; Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA |
Аффилиация |
Huang, Q.; NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, USA |
Аффилиация |
Lynn, J. W.; NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, USA |
Аффилиация |
Li, Jiying; NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, USA; Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742-6393, USA |
Аффилиация |
II, W. Ratcliff; NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, USA |
Аффилиация |
Zarestky, J. L.; Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, USA |
Аффилиация |
Mook, H. A.; Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA |
Аффилиация |
Chen, G. F.; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China |
Аффилиация |
Luo, J. L.; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China |
Аффилиация |
Wang, N. L.; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China |
Аффилиация |
Dai, Pengcheng; Department of Physics and Astronomy, The University of Tennessee, Knoxville, Tennessee 37996-1200, USA; Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA |
Выпуск |
7197 |